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Axion-like particles (ALPs) arise from well-motivated extensions to the Standard Model and could account for dark matter. ALP dark matter would manifest as a field oscillating at an (as of yet) unknown frequency. The frequency depends linearly on the ALP mass and plausibly ranges from 10⁻²²to 10 eV/c². This motivates broadband search approaches. We report on a direct search for ALP dark matter with an interferometer composed of two atomic K-Rb-³He comagnetometers, one situated in Mainz, Germany, and the other in Kraków, Poland. We leverage the anticipated spatio-temporal coherence properties of the ALP field and probe all ALP-gradient-spin interactions covering a mass range of nine orders of magnitude. No significant evidence of an ALP signal is found. We thus place new upper limits on the ALP-neutron, ALP-proton and ALP-electron couplings reaching belowg_aNN < 10⁻⁹ GeV⁻¹,g_aPP < 10⁻⁷ GeV⁻¹andg_aee < 10⁻⁶ GeV⁻¹, respectively. These limits improve upon previous laboratory constraints for neutron and proton couplings by up to three orders of magnitude. 

We search for dark matter in the form of axionlike particles (ALPs) in the mass range $5.576741\mathrm{neV}/{\mathrm{c}}^2-5.577733\mathrm{neV}/{\mathrm{c}}^2$by probing their possible coupling to fermion spins through the ALP field gradient. This is achieved by performing proton nuclear magnetic resonance spectroscopy on a sample of methanol as a technical demonstration of the Cosmic Axion Spin Precession Experiment Gradient (CASPEr-Gradient) Low-Field apparatus. Searching for spin-coupled ALP dark matter in this mass range with associated Compton frequencies in a 240 Hz window centered at 1.348570 MHZ resulted in a sensitivity to the ALP-proton coupling constant of $g_{\mathrm{ap}}\approx 3\times {10}^{-2}{\mathrm{GeV}}^{-1}$. This narrow-bandwidth search serves as a proof-of-principle and a commissioning measurement, validating our methodology and demonstrating the experiment’s capabilities. CASPEr-Gradient Low-Field will probe the mass range from $4.1\mathrm{peV}/{\mathrm{c}}^2$to $17\mathrm{neV}/{\mathrm{c}}^2$with hyperpolarized samples to boost the sensitivity beyond the astronomical limits. 

Abstract Numerous theories extending beyond the standard model of particle physics predict the existence of bosons that could constitute dark matter. In the standard halo model of galactic dark matter, the velocity distribution of the bosonic dark matter field defines a characteristic coherence time τ c . Until recently, laboratory experiments searching for bosonic dark matter fields have been in the regime where the measurement time T significantly exceeds τ c , so null results have been interpreted by assuming a bosonic field amplitude Φ 0 fixed by the average local dark matter density. Here we show that experiments operating in the T  ≪  τ c regime do not sample the full distribution of bosonic dark matter field amplitudes and therefore it is incorrect to assume a fixed value of Φ 0 when inferring constraints. Instead, in order to interpret laboratory measurements (even in the event of a discovery), it is necessary to account for the stochastic nature of such a virialized ultralight field. The constraints inferred from several previous null experiments searching for ultralight bosonic dark matter were overestimated by factors ranging from 3 to 10 depending on experimental details, model assumptions, and choice of inference framework. 

Abstract Hidden matter that interacts only gravitationally would oscillate at characteristic frequencies when trapped inside of Earth. For small oscillations near the center of the Earth, these frequencies are around 300 μHz. Additionally, signatures at higher harmonics would appear because of the non-uniformity of Earth’s density. In this work, we use data from a global network of gravimeters of the International Geodynamics and Earth Tide Service (IGETS) to look for these hypothetical trapped objects. We find no evidence for such objects with masses on the order of 10 14  kg or greater with an oscillation amplitude of 0.1 r e . It may be possible to improve the sensitivity of the search by several orders of magnitude via better understanding of the terrestrial noise sources and more advanced data analysis. Graphical abstract 

The nature of dark matter, the invisible substance making up over 80% of the matter in the universe, is one of the most fundamental mysteries of modern physics. Ultralight bosons such as axions, axion-like particles, or dark photons could make up most of the dark matter. Couplings between such bosons and nuclear spins may enable their direct detection via nuclear magnetic resonance (NMR) spectroscopy: As nuclear spins move through the galactic dark-matter halo, they couple to dark matter and behave as if they were in an oscillating magnetic field, generating a dark-matter–driven NMR signal. As part of the cosmic axion spin precession experiment (CASPEr), an NMR-based dark-matter search, we use ultralow-field NMR to probe the axion-fermion “wind” coupling and dark-photon couplings to nuclear spins. No dark matter signal was detected above background, establishing new experimental bounds for dark matter bosons with masses ranging from 1.8 × 10 −16 to 7.8 × 10 −14 eV.